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A LA-ICP-MS sulphide calibration standard based on a chalcogenide glass
Journal article   Peer reviewed

A LA-ICP-MS sulphide calibration standard based on a chalcogenide glass

L. Ding, G. Yang, F. Xia, C.E. Lenehan, G. Qian, A. McFadden, J.L. Brugger, X. Zhang, G. Chen and A. Pring
Mineralogical Magazine, Vol.75(2), pp.279-287
2011
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Abstract

The accurate measurement of trace element concentrations in natural sulphides by laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS) has been limited by the lack of matrix-matched calibration standards. The synthesis of a standard, IMER-1, by incorporating four minor and 34 trace elements into a chalcogenide glass matrix Ge28Sb12S60 is reported here. Chemical analysis by electron probe microanalysis (EPMA), LA-ICP-MS, solution ICP-MS, and inductively coupled plasma-optical emission spectroscopy (ICP-OES) confirmed the excellent homogeneity of major elements (1-σ relative standard deviation (RSD) <1% for S, Sb and Ge) and acceptable homogeneity of most trace elements (1-σ RSD <10%). The standard was validated by analysing trace-elements concentrations in three geological pyrite specimens using IMER-1 as the calibration standard and comparing the results to previously reported values also determined by LA-ICP-MS but using a different calibration standard, STDGL2b-2. The results suggest that IMER-1 may be an appropriate calibration standard for LA-ICP-MS analysis of trace elements in natural sulphides.

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Collaboration types
Domestic collaboration
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Citation topics
8 Earth Sciences
8.8 Geochemistry, Geophysics & Geology
8.8.1 Geochemical Petrogenesis
Web Of Science research areas
Mineralogy
ESI research areas
Geosciences
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