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Carbonic anhydrase inhibitors — Part 47: Quantum chemical quantitative structure-activity relationships for a group of sulfanilamide Schiff base inhibitors of carbonic anhydrase
Journal article   Peer reviewed

Carbonic anhydrase inhibitors — Part 47: Quantum chemical quantitative structure-activity relationships for a group of sulfanilamide Schiff base inhibitors of carbonic anhydrase

C.T. Supuran and B.W. Clare
European Journal of Medicinal Chemistry, Vol.33(6), pp.489-500
06/1998
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Abstract

A series of sulfanilamide Schiff base inhibitors of CA I and CA II have been studied by the semi-empirical AM1 method. The charges on the atoms of the sulfonamide group, and the dipole moment, have been calculated by four methods: a standard vacuum calculation, a solution calculation by the COSMO method, a solution calculation with, in addition, the charges and dipole moments calculated by fitting to the calculated electrostatic potential, and a calculation by the older CNDO method. The data were subjected to a classical multiple regression analysis with care to avoid the possibility of chance correlation or collinearity. The ACE technique was also used to allow for nonlinearity. A number of statistically significant equations were derived, which were mostly consistent with previous studies. While the ESP-based charges gave the best equations, the improvement was not sufficient to convincingly exclude the other methods. This is the first study which evidenced by means of QSAR calculations isozyme-specific features of the two isozymes CA I and CA II, in their interaction with sulfonamide inhibitors.

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Collaboration types
Domestic collaboration
International collaboration
Citation topics
2 Chemistry
2.123 Protein Stucture, Folding & Modelling
2.123.1896 Carbonic Anhydrase Inhibitors
Web Of Science research areas
Chemistry, Medicinal
ESI research areas
Chemistry
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