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Conversion of fluorine-containing ozone-depleting and greenhouse gases to valuable polymers in a nonthermal plasma
Journal article   Peer reviewed

Conversion of fluorine-containing ozone-depleting and greenhouse gases to valuable polymers in a nonthermal plasma

E.M. Kennedy, S.K. Kundu, J.C. Mackie, C.I. Holdsworth, T.S. Molloy, V.V. Gaikwad and B.Z. Dlugogorski
Industrial & Engineering Chemistry Research, Vol.51(34), pp.11279-11283
2012
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Abstract

A dielectric barrier discharge (DBD) nonthermal plasma was used to convert a range of fluorocarbons into useful polymeric products. Reactions were conducted at atmospheric pressure, in an argon bath gas and where methane was added as reactant. The bulk gas temperature was less than 150 °C and yielded polymers from a number of methane/fluorocarbon mixtures, including fluorocarbons such as halons, chlorofluorocarbons (CFCs), hydrochlorofluorocarbons (HCFCs), hydrofluorocarbons (HFCs), and perfluorocarbons (PFCs). The results of gel permeation chromatography (GPC) reveal that a potentially valuable polymer is synthesized, with a number average molecular weight of between 60 000 and 130 000 g mol -1 and a polydispersity index (PDI) of between 1.2 and 2.9, depending on the fluorochemical converted.

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Citation topics
5 Physics
5.202 Plasma Physics
5.202.388 Plasma Discharges
Web Of Science research areas
Engineering, Chemical
ESI research areas
Chemistry
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