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High temperature in-situ phase stability of sputtered TiAlxN coatings
Journal article   Open access   Peer reviewed

High temperature in-situ phase stability of sputtered TiAlxN coatings

S.B. Patel, E. Mohammadpour, N. Mondinos, X. Zhao, J-P Veder, Z. Zhou, T.S.Y. Moh, W.Y. Hsien Liew, S. Lee and Z-T Jiang
Journal of Alloys and Compounds, Vol.786, pp.507-514
2019
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Abstract

The temperature dependence of phase composition and lattice parameters, for TiAlxN thin film coating, are experimentally investigated by in-situ synchrotron radiation X-ray diffraction (SR-XRD), at temperatures between 25 °C and 700 °C. Mechanical properties, such as: Young's modulus (E), hardness (H) and plastic deformation index (PDI) – were experimentally determined by nanoindentation, at 25 °C. Crystalline structural analysis, of SR-XRD results, indicates the major phases are TiN and AlN; with Ti2O and TiO2 phases also present above 600 °C. The lattice constants increased with an increase in temperature. Atomic and phase compositions, at 25 °C, were also verified by X-ray photoelectron spectroscopy (XPS). Field emission scanning electron microscopy (FESEM) images display an increase in surface roughness and reduction in grain size, with increasing Aluminium percentage (Al%). Nanoindentation analysis showed a maximum hardness of 25.1 ± 1.5 GPa (sample containing 12% Al), which was subsequently reduced upon addition of more Aluminium. Finite element modelling (FEM), including von Mises stress distribution, indicates lower mechanical integrity, for samples with high Al% content.

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Collaboration types
Domestic collaboration
International collaboration
Citation topics
5 Physics
5.188 Deposition, Hardening & Coating
5.188.318 Nitride Coatings
Web Of Science research areas
Chemistry, Physical
Materials Science, Multidisciplinary
Metallurgy & Metallurgical Engineering
ESI research areas
Materials Science
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