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Singlet-diradical character in large PAHs triggers spontaneous-ignition of coal
Journal article   Peer reviewed

Singlet-diradical character in large PAHs triggers spontaneous-ignition of coal

M. Altarawneh, I. Oluwoye and B.Z. Dlugogorski
Combustion and Flame, Vol.212, pp.279-281
2020
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Abstract

Chemical phenomena dictating the spontaneous-ignition of coal remain highly speculative with some of the most intriguing questions appearing unaddressed. In this communication, we deploy a synergistic experimental-theoretical approach to elucidate the definite role of singlet-biradical PAHs in driving the low-temperature oxidation of coal. We establish that, five linearly-fused benzene rings (i.e., pentacene, as a model compound for the PAH content in coal, and an example of short-chain graphene nanoribbons) ignites 200 °C lower than the corresponding temperature for naphthalene.

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Collaboration types
Domestic collaboration
International collaboration
Citation topics
7 Engineering & Materials Science
7.139 Energy & Fuels
7.139.1964 Spontaneous Combustion
Web Of Science research areas
Energy & Fuels
Engineering, Chemical
Engineering, Mechanical
Engineering, Multidisciplinary
Thermodynamics
ESI research areas
Engineering
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