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Solid-solute phase equilibria in aqueous solution. IV. Calculation of Phase Diagrams
Journal article   Peer reviewed

Solid-solute phase equilibria in aqueous solution. IV. Calculation of Phase Diagrams

E. Königsberger and H. Gamsjäger
Zeitschrift für anorganische und allgemeine Chemie, Vol.584(1), pp.185-193
1990
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Abstract

The thermodynamic principles of conventional (T-x, P-T) phase diagrams and solubility (log ΣK-x) diagrams depicting solid-solute phase equilibria in aqueous solution are derived from a unifying point of view. It is shown that thermodynamic quantities necessary for the construction of conventional phase diagrams can be obtained from solubility measurements. The unary system calcite-aragonite and the binary system aragonite-strontianite, where solubility data are available over the whole compositional range, have been selected as examples. In the latter case, the constraint of constant composition of the solid phase leading to a metastable equilibrium with the respective solute species is an essential point in the thermodynamic derivation and was observed experimentally as well.

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Web Of Science research areas
Chemistry, Inorganic & Nuclear
ESI research areas
Chemistry
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