Logo image
The non-oxidative dissolution of nickel sulphides in aqueous acidic solutions
Journal article   Open access   Peer reviewed

The non-oxidative dissolution of nickel sulphides in aqueous acidic solutions

A.O. Filmer and M.J. Nicol
Journal of the South African Institute of Mining and Metallurgy, Vol.80(12), pp.415-424
1980
pdf
nickel sulphides.pdfDownloadView
Published (Version of Record) Open Access

Abstract

An account is given of a study on the non-oxidative dissolution in aqueous acidic solutions of nickel sulphides of different stoichiometric composition, in which a rotating ring-disc electrode was used. The rate of dissolution was found to depend on the potential of the sulphide and the nickel-to-sulphur stoichiometric ratio. A maximum rate for the dissolution of nickel from nickel sulphides containing an excess of nickel was recorded at potentials around -0,2 to -O,3V. The rate decreased markedly at more anodic potentials. For nickel-deficient nickel sulphides, the nonoxidative dissolution rate increased with a cathodic shift in potential. Under open-circuit conditions, a nickel sulphide of a composition approximating Ni ,S. reacted most rapidly. The dissolution rate was controlled by either a chemical or an electrochemical reaction at the electrode surface, had an activation energy of between 50 and 65 kJ.mol-1, and was independent of stirring speed.

Details

Metrics

116 File views/ downloads
55 Record Views
Logo image